Homogeneous Catalytic Dimerization of Terminal Alkynes by C5Me5Ru(L)H3 (L = PPh3, PCy3, PMe3)

The ruthenium hydride complexes C5Me5Ru(L)H3, PCy3, PMe3 ) were found to catalyze the dimerization reaction of terminal alkynes RC⋮CH to produce cis- and trans-1,4-disubstituted enynes RCHCHC⋮CR and 1,3-disubstituted enynes CH2C(R)C⋮CR

Chae S. Yi; Nianhong Liu

2002

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  • The ruthenium hydride complexes C5Me5Ru(L)H3, PCy3, PMe3) were found to catalyze the dimerization reaction of terminal alkynes RC⋮CH to produce cis- and trans-1,4-disubstituted enynes RCHCHC⋮CR and 1,3-disubstituted enynes CH2C(R)C⋮CR
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  • A mechanistic interpretation is presented on the basis of the product distribution
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