Overcoming the Rate-Limiting Reaction during Photoreforming of Sugar Aldoses for H2-Generation

We identified that this decrease is due to kinetic constraints rather than to catalyst deactivation

Kai E. Sanwald; Tobias F. Berto; Wolfgang Eisenreich; Andreas Jentys; Oliver Y. GutiƩrrez; Johannes A. Lercher

2017

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  • Photoreforming of sugars on metalloaded semiconductors is an attractive process for H2-generation
  • The nature of the rate-limiting reaction was elucidated by investigation of the reaction pathways and oxidation mechanisms during photoreforming of sugar aldoses on TiO2 decorated with Rh, Pd, or Pt
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